DOI > 10.5291/ILL-DATA.4-02-510

This proposal is publicly available since 04/23/2023

Title

Spin-space anisotropy of magnetic excitations in FeSe(1-x)S(x)

Abstract

Understanding the microscopic mechanism of superconductivity in iron-based materials is one of the most important quests in condensed matter physics research. While most theories have assumed an insignificant role of spin-orbit coupling, recent ARPES experiments showed that the energy scale of spin-orbit coupling might have been underestimated. In our recent study of FeSe(1-x)S(x) for x=0 and 0.07, we have indeed observed distinct spin-space anisotropy in the low-energy magnetic excitations, which clearly demonstrates that spin-orbit coupling casts a substantial influence on the magnetism, and that the presence of spin-space anisotropy does not require long-range magnetic order. Here, we propose to use spin-polarized inelastic neutron scattering to further pursue the study of spin-space anisotropy of magnetic excitations up to higher sulfur concentrations towards x=0.20, where a nematic quantum critical point may exist, in order to elucidate the relation between spin-orbit coupling, the nematic order, and the optimization of superconductivity.

Experimental Report

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Data Citation

The recommended format for citing this dataset in a research publication is in the following format:

LI Yuan; BOURDAROT Frederic; Bourges; JEONG Jaehong; Mingwei MA; SIDIS Yvan and Guoqing Wang. (2018). Spin-space anisotropy of magnetic excitations in FeSe(1-x)S(x). Institut Laue-Langevin (ILL) doi:10.5291/ILL-DATA.4-02-510

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Metadata

Experiment Parameters

  • Environment temperature

    1.5-300K
  • Experiment energy

    2meV<w<10meV,kf=2.66
  • Experiment moment

    0.7 - 1.6 A^-1
  • Experiment res energy

    1meV (or standard)
  • Experiment res moment

    standard

Sample Parameters

  • Formula

    • FeSe(0.8)S(0.2)
    • FeSe(0.85)S(0.15)