Study of the porous structure of pure and N-functionalised zeolite-templated carbons
Development of high efficiency and safe hydrogen storage materials is vital for the move towards a hydrogen based greenhouse gas emission free and sustainable economy. Zeolite-templated carbons are a class of highly potential hydrogen storage materials. In addition, the highly ordered microporous structure of zeolite-templated carbons is excellent as a model material to investigate the hydrogen-carbon interactions in pores with specific sizes, geometries, and with chemical dopants. In this study we apply to characterise the porosity of three high surface are microporous zeolite-templated carbons. Two of the zeolite-templated carbons have been functionalised with N-groups to investigate the hydrogen interactions with N-functionalised ordered microporous carbon structures in complementary lab-scale and SANS and ND measurements. Deuterated toluene contrast-matched SANS will be used to subtract the signal from closed porosity and density fluctuations from inside the carbon material and to determine the prevalent structure of partially filled porosity. This measurement will yield highly valuable characterisation of the porous structure of materials of high interest.
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Rasmus Palm; CUBITT Robert; ELSON Frank; Ola Kenji Forslund; Yuqing Ge; HARMAS Riinu; KORJUS Ove; MANSSON MARTIN; Ugne Miniotaite; NOCERINO Elisabetta; OSUAGWU Emmanuel; Yasmine Sassa and TUUL Kenneth. (2023). Study of the porous structure of pure and N-functionalised zeolite-templated carbons. Institut Laue-Langevin (ILL) doi:10.5291/ILL-DATA.6-07-106
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