Confined crystalline D2 phase in ordered microporous zeolite-templated carbons
Development of high efficiency and safe hydrogen storage materials is vital for the move towards a hydrogen based greenhouse gas emission free and sustainable economy. Zeolite-templated carbons are a highly potential hydrogen storage materials. In addition, the highly ordered microporous structure of zeolite-templated carbons (ZTC) is excellent as a model material to investigate the hydrogen-carbon interactions in pores with specific sizes, geometries, and also chemical makeups. In this study we will determine the influence of the ordered microporus carbon structure on the D2 crystallisation. For this three ZTCs are used, where the influence of N-functionalisation is investigated via two samples, which have been prepared to contain N-functionalisations. The adsorbent porosity influence on melting temperature and the crystalline fine-structure will be determined. This study is planned in tandem with SANS and QENS measurements to form a complete picture about the H2-carbon interactions in case of N-functionalised ZTCs.
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Rasmus Palm; ELSON Frank; Ola Kenji Forslund; Yuqing Ge; Thomas C. Hansen; HARMAS Riinu; KORJUS Ove; MANSSON MARTIN; Ugne Miniotaite; MOLLER Egert; NOCERINO Elisabetta; OSUAGWU Emmanuel and Yasmine Sassa. (2023). Confined crystalline D2 phase in ordered microporous zeolite-templated carbons. Institut Laue-Langevin (ILL) doi:10.5291/ILL-DATA.6-07-107
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