Study of H2 mass transport and dynamics in ordered microporous zeolite-templated carbons
Development of high efficiency and safe hydrogen storage materials is vital for the move towards a hydrogen-based greenhouse gas emission free and sustainable economy. Zeolite-templated carbons (ZTCs) are a class of highly potential hydrogen storage materials. In addition, the highly ordered microporous structure of ZTCs is excellent as a model material to investigate the hydrogen-carbon interactions in pores with specific sizes, geometries, and with chemical dopants. In this study we propose to investigate the influence of the ordered microporous ZTC structures and N-functionalisation of these structures on the hydrogen mass transport properties. The hydrogen mass transport and dynamic properties will be determined from the quasi-elastic broadening of H2 neutron scattering. From this the influence of N-functionalise groups on H2 confinement in the porous structure will be determined. The H2 transport properties will be collaborated with the porous structure characterisation applied for on SANS instrument D33 and with lab-scale characterisation.
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Rasmus Palm; ELSON Frank; Ola Kenji Forslund; Yuqing Ge; HARMAS Riinu; KOPPEL Miriam; KORJUS Ove; MANSSON MARTIN; Ugne Miniotaite; NOCERINO Elisabetta; OLLIVIER Jacques; OSUAGWU Emmanuel and Yasmine Sassa. (2023). Study of H2 mass transport and dynamics in ordered microporous zeolite-templated carbons. Institut Laue-Langevin (ILL) doi:10.5291/ILL-DATA.6-07-108
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