DOI > 10.5291/ILL-DATA.7-05-550

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Title

Proving the existence of high temperature, intermolecular nuclear magnetic ordering in nanoconfined H2

Abstract

Magnetic nuclear spin correlations between nuclei are very rare in materials, typically only occurring at very low temperatures (nK-mK). These coherent quantum phases of matter are of particular interest as quantum sensors or even as neutron polarizer materials. We have collected preliminary data indicating long-range nuclear spin coupling may occur for nanoconfined hydrogen molecules (H2) at temperatures 3-4 orders of magnitude higher than the current record. Using temperature-dependent XYZ spin polarised neutron scattering on WASP, these experiments will decouple nuclear spin-incoherent, nuclear coherent and magnetic scattering of nanoconfined H2 to experimentally determine if previously observed scattering deviations are indeed caused by intermolecular (H2-H2) nuclear-spin correlations or alternatively originate from nuclear short-range order between H2 and C or electronic magnetic interactions with the carbon network. If nuclear spin correlations between nanoconfined H2 molecules are proven, this work will demonstrate how coherent quantum phases of matter can be generated at temperatures far higher than the current state of the art using a simple methodology ¿ nanoconfinement.

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Data Citation

The recommended format for citing this dataset in a research publication is in the following format:

Lui R. Terry; FALUS Peter; FOUQUET Peter; ROLS Stephane; TING Valeska and WILDES Andrew. (2023). Proving the existence of high temperature, intermolecular nuclear magnetic ordering in nanoconfined H2. Institut Laue-Langevin (ILL) doi:10.5291/ILL-DATA.7-05-550

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